当前位置：首页>武汉>武汉工程大学秦平力&湖北科技学院Zhonli Qin团队最新AFM:富氧分子桥接界面实现高性能钙钛矿太阳电池

武汉工程大学秦平力&湖北科技学院Zhonli Qin团队最新AFM:富氧分子桥接界面实现高性能钙钛矿太阳电池

  • 2026-10-08 20:01:16
武汉工程大学秦平力&湖北科技学院Zhonli Qin团队最新AFM:富氧分子桥接界面实现高性能钙钛矿太阳电池
埋底界面缺陷以及能级失配是钙钛矿太阳电池（PSCs）面临的主要挑战，它们会形成严重非辐射复合的退化中心，从而限制器件性能。
基于此，武汉工程大学秦平力&湖北科技学院Zhonli Qin团队将双草酸硼酸锂（LiBOB）引入电子传输层（ETL）/钙钛矿界面，相关成果发表于Advanced Functional Materials期刊。作为一种多功能路易斯碱，高极性的BOB−阴离子能够与路易斯酸性的Pb2+和Sn4+发生配位作用。该相互作用可促进钙钛矿前驱体薄膜形成均匀的异质成核，从而获得更大的钙钛矿晶粒，并有效降低体相及晶界缺陷。
与此同时，LiBOB还能有效调节SnO2量子点电子传输层的能带结构，实现钙钛矿与SnO2量子点ETL之间更有利的能级匹配，从而降低界面势垒，促进电子的顺畅传输与提取。因此，基于LiBOB的钙钛矿太阳电池实现了26.15%的冠军光电转换效率。在环境条件下储存3600小时后，该器件仍保持约91%的初始效率，显著优于对照器件（仅保留53%的初始效率）。
论文信息：B. Yuan, J. He, B. Ding, et al. “ Oxygen-Rich Molecular Bridging Interface Enable High-Performance Perovskite Solar Cells.” Advanced Functional Materials (2026): e75843. https://doi.org/10.1002/adfm.75843
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